Low-dimensional Magnetism in Novel 2D Honeycomb Materials

Sammanfattning: A Kitaev quantum spin liquid is a phase of matter predicted to host excitations that can be used to preform fault-tolerant quantum computation. Though the theoretical prediction of such a state is on firm footing, its realisation in real materials has proven to be elusive. Recent developments have suggested honeycomb materials consisting of 3d transition metal ions as possible candidates. The focus of this thesis is the magnetic properties of one such material, K2Ni2–xCoxTeO6. It is part of a family of layered two dimensional materials consisting of honeycomb structured transition metal layers sandwiched between layers of alkali ions. A characterisation of the magnetic properties of K2Ni2–xCoxTeO6 has been carried out with the techniques of muon spin rotation/relaxation/resonance and bulk magnetisation as a function of the chemical composition. Further investigations of the detailed atomic structure and spin order using neutron scattering was also initiated. The results of such characterisations are presented and discussed in this thesis.